Chirped pulse amplification

Stretcher and compressor design

There are several ways to construct compressors and stretchers. However, a typical Ti:sapphire-based chirped-pulse amplifier requires that the pulses are stretched to several hundred picoseconds, which means that the different wavelength components must experience about 10 cm difference in path length. The most practical way to achieve this is with grating-based stretchers and compressors. Stretchers and compressors are characterized by their dispersion. With negative dispersion, light with higher frequencies (shorter wavelengths) takes less time to travel through the device than light with lower frequencies (longer wavelengths). With positive dispersion, it is the other way around. In a CPA, the dispersions of the stretcher and compressor must cancel out. Because of practical considerations, the (high-power) compressor is usually designed with negative dispersion, and the (low-power) stretcher is therefore designed with positive dispersion.

In principle, the dispersion of an optical device is a function ${\displaystyle \tau (\omega )}$, where ${\displaystyle \tau }$ is the time delay experienced by a frequency component ${\displaystyle \omega }$. (Sometimes the phase ${\displaystyle \varphi (\omega )=2\pi \tau (\omega )c/\lambda (\omega )}$ is used, where c is the speed of light and ${\displaystyle \lambda }$ is the wavelength.) Each component in the whole chain from the seed laser to the output of the compressor contributes to the dispersion. It turns out to be hard to tune the dispersions of the stretcher and compressor such that the resulting pulses are shorter than about 100 femtoseconds. For this, additional dispersive elements may be needed.

With gratings

Figure 1 shows the simplest grating configuration, where long-wavelength components travel a larger distance than the short-wavelength components (negative dispersion). Often, only a single grating is used, with extra mirrors such that the beam hits the grating four times rather than two times as shown in the picture.

This setup is normally used as a compressor since it does not involve transmissive components that could lead to unwanted side-effects when dealing with high-intensity pulses. The dispersion can be tuned easily by changing the distance between the two gratings. The introduced dispersion by such a compressor is often described in dispersion orders: the group delay dispersion (GDD), third order of dispersion (TOD) etc. Figure 2 shows the dispersion orders for a grating compressor with a groove density of ${\displaystyle \sigma =1700\mathrm{l}\mathrm{i}\mathrm{n}\mathrm{e}\mathrm{s}/\mathrm{m}\mathrm{m}}$, an incidence angle of ${\displaystyle {\theta }_{in}={65}^{\circ }}$, and a normal grating separation of ${\displaystyle L=25\mathrm{c}\mathrm{m}}$, as described in the original design by Donna Strickland and Gérard Mourou (1985), and evaluated using Lah-Laguerre optical formalism - a generalized formulation of the high orders of dispersion.

Figure 3 shows a more complicated grating configuration that involves focusing elements, here depicted as lenses. The lenses are placed at a distance ${\displaystyle 2f}$ from each other (they act as a 1:1 telescope), and at a distance ${\displaystyle L}$ from the gratings. If ${\displaystyle L<f}$, the setup acts as a positive-dispersion stretcher and if ${\displaystyle L>f}$, it is a negative-dispersion stretcher. The ${\displaystyle L=f}$ case is used in femtosecond pulse shaping. Usually, the focusing element is a spherical or cylindrical mirror rather than a lens. As with the configuration in Figure 1, it is possible to use an additional mirror and use a single grating rather than two separate ones. This setup requires that the beam diameter is very small compared to the length of the telescope; otherwise undesirable aberrations will be introduced. For this reason, it is normally used as a stretcher before the amplification stage, since the low-intensity seed pulses can be collimated to a beam with a small diameter.

With prisms

It is possible to use prisms rather than gratings as dispersive elements, as in Figure 4. Despite such a simple change, the set-up behaves quite differently, as to first order no group delay dispersion is introduced. Such a stretcher/compressor can have both a positive or negative dispersion, depending on the geometry and the material properties of the prisms. With lenses, the sign of the dispersion can be reversed, similar to Figure 3. For a given distance between the dispersive elements, prisms generate much less dispersion than gratings. Prisms and gratings are sometimes combined to correct higher order dispersion ("grisms"), in which case the distance between the prisms is on the order of 10 meters rather than 50 cm as with a grating compressor. Gratings lose power into the other orders, while prisms lose power due to Rayleigh scattering. As an example, the dispersion orders of a fused silica prism-pair compressor are illustrated in Figure 5 for variable insertion depth of the first prism ${\displaystyle {\ell }_1}$. The dispersion is evaluated for laser pulses at ${\displaystyle 780\text{ nm}}$ with spectral bandwidth of ${\displaystyle \mathrm{\Delta }\lambda =30\text{ nm}}$, using Lah-Laguerre optical formalism - a generalized formulation of the high orders of dispersion. The compressor parameters at near Brewster incidence angle are: normal distance between the prisms of ${\displaystyle L=30\text{ cm}}$, insertion depth of the second prism ${\displaystyle {\ell }_2=\text{1 mm}}$ at ${\displaystyle {\lambda }_{min}}$ and an apex angle of the fused silica prisms ${\displaystyle \alpha ={69.06}^{\circ }}$. The particular values depend on the prism material, the wavelength of interest as well as on the compressor parameters.

Phase conjugation of chirped pulses

Chirped pulses from ${\displaystyle N}$ laser amplifiers may be phase locked via reflection from a phase-conjugating mirror to increase the brightness as ${\displaystyle N^2}$. For this purpose degenerate four-wave mixing Kerr phase conjugation is relevant.

Other techniques

Some other techniques can be used for stretching and compressing pulses, but these are not suitable as the main stretcher/compressor in CPA due to their limited amount of dispersion and due to their inability to handle high-intensity pulses.

• A pulse can be stretched simply by letting it propagate through a thick slab of transparent material, such as 200 mm glass. As with the prisms, only a limited amount of dispersion can be achieved within physically practical dimensions. Outside the visible-light spectrum, materials exist both for positive and negative dispersion. For visible and near-infrared wavelengths, almost all transparent materials have positive dispersion. However, glass fibres can have their dispersion tailored to meet the needs.
• One or multiple reflections between a pair of chirped mirrors or similar device allow any form of chirp. This is often used in conjunction with the other techniques to correct for higher orders.
• The Dazzler is a commercial pulse shaper in which light is diffracted from an acoustic wave. By tuning the timing, frequency, and amplitude of the acoustic wave, it is possible to introduce arbitrary dispersion functions with a maximum delay of a few picoseconds.
• A phase-shifting mask can be placed in the focal plane of the stretcher in Fig. 3, which introduces additional dispersion. Such a mask can be an LCD array, where the phase shift can be tuned by changing the voltage on the pixels. This can generate arbitrary dispersion functions with a maximum of a few tens of picoseconds of delay. Such a setup is called a pulse shaper.

Applications

CPA is used in all of the highest-power lasers (greater than about 100 terawatts) in the world, with the exception of the ≈500 TW National Ignition Facility. Some examples of these lasers are the Vulcan laser at the Rutherford Appleton Laboratory's Central Laser Facility, the Diocles laser at the University of Nebraska–Lincoln, the GEKKO XII laser at the GEKKO XII facility in the Institute for Laser Engineering at Osaka University, the OMEGA and OMEGA EP lasers at the University of Rochester's Lab for Laser Energetics and the now dismantled petawatt line on the former Nova laser at the Lawrence Livermore National Laboratory. Gérard Mourou has proposed using CPA to generate high-energy and low-duration laser pulses to transmute highly radioactive material (contained in a target) to significantly reduce its half-life, from thousands of years to only a few minutes.

Apart from these state-of-the-art research systems, a number of commercial manufacturers sell Ti:sapphire-based CPAs with peak powers of 10 to 100 gigawatts.